A　self-assembled　Cu-Fe-Ni-Cr-Si　immiscible　composite　with　a　bilayer　structure　was　produced　by　laser　induction　hybrid　cladding　(LIHC)　as　a　result　of　liquid　phase　separation　(LPS).　The　microstructure　exhibited　by　large　amounts　of　ferromagnetic　(FM)　Fe3Si　particles　dispersed　within　the　epsilon-Cu　matrix　in　the　upper　layer,　and　many　epsilon-Cu　particles　embedded　within　the　FM　Fe3Si　matrix　in　the　lower　layer.　The　microhardness　values　of　the　Fe3Si　matrix　lower　layer　(758HV(0.2))　and　epsilon-Cu　matrix　upper　layer　(248HV(0.2))　were　similar　to　7.3　and　similar　to　2.4　times　higher　than　that　of　pure　copper　by　LIHC,　respectively,　indicating　that　the　immiscible　composite　exhibited　strongly　inhomogeneous　characteristics　consistent　with　a　＂bilayer　structure＂.　Moreover,　the　immiscible　composite　showed　a　high　saturation　magnetization　of　96.2　emu/g　and　a　low　coercivity　of　7.24　Oe　due　to　the　formation　of　FM　Fe3Si　with　micro-and　nanoscaled　structures.　(c)　2018　Elsevier　B.V.　All　rights　reserved.