Developing　advanced　lithium-ion　batteries　that　afford　both　high　energy　density　and　high　power　density　has　been　one　of　the　crucial　research　targets　in　the　field　of　electrochemical　energy　storage.　Realization　of　fast　Li+　storage　would　require　a　smart　electrode　design　that　enables　simultaneous　enhancements　in　ion　and　electron　transports　as　well　as　a　fast　and　facile　bulk-form　solid-state　reaction.　Here　we　report　a　high-performance　3D　bilayered　composite　electrode　constructed　by　bicontinuous　nanoporous　graphene　and　thin　molybdenum　oxide　stacking　films.　The　novel　electrode　offers　fast　kinetics　of　Li+　diffusion　and　reactions　and,　consequently,　delivers　a　large　specific　capacity　of　710　mAh　g(-1),　the　excellent　rate　performance　of　charging　within　seconds　and　an　ultra-long　lifetime　over　13,000　discharge-charge　cycles.　High　and　stable　volumetric　capacities　up　to　900　mAh　cm(-3)　have　also　been　achieved　with　the　squeezed　composite　electrodes.　This　study　shines　light　into　the　realization　of　a　high-performance　graphene-based　porous　electrode　for　advanced　lithium-ion　batteries　and　will　inspire　the　development　of　new　3D　hybrid　materials　for　high-rate　and　large-capacity　electrochemical　energy　storage.