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作者:

Liang, Wen-Jun (Liang, Wen-Jun.) (学者:梁文俊) | Ren, Si-da (Ren, Si-da.) | Li, Yu-ze (Li, Yu-ze.) | Shi, Xiu-juan (Shi, Xiu-juan.) | Li, Jian (Li, Jian.)

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SCIE

摘要:

A catalytic reverse flow reactor was employed for the combustion of lean carbon monoxide in air mixture. The catalytic combustion of CO over a Pd mixed oxide supported on cordierite coated with Ce/La was investigated. The catalysts were prepared using a sol-gel method and characterized using BET and SEM. The effects of Pd content, preheated temperature, calcination temperature and calcination time on catalyst performance were studied. Furthermore, the performances of the reactor such as pressure drop and bed temperature distribution were investigated. The catalysts calcined at 550 degrees C for 3 h with Pd content being 2.5 wt% exhibited the highest catalytic activity. The conversion attained 90% when the switch time was 8 min, the GHSV was 8000h(-1), and the initial concentration was 100ppm. The pressure drop of the system was small when the GHSV was lower than 10000h(-1). The initial preheating temperature of the catalyst had a greater influence on the temperature distribution in the reactor.

关键词:

rare earth metal reverse flow catalytic combustion Pd monolithic catalyst Carbon monoxide

作者机构:

  • [ 1 ] [Liang, Wen-Jun]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 2 ] [Ren, Si-da]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 3 ] [Li, Yu-ze]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 4 ] [Shi, Xiu-juan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 5 ] [Li, Jian]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

通讯作者信息:

  • 梁文俊

    [Liang, Wen-Jun]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

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来源 :

FRESENIUS ENVIRONMENTAL BULLETIN

ISSN: 1018-4619

年份: 2018

期: 12

卷: 27

页码: 8297-8307

ESI学科: ENVIRONMENT/ECOLOGY;

ESI高被引阀值:203

JCR分区:4

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