Flaky　FeSiAl　alloy　(9.5　wt%　Si,　5.5　wt%　Al　and　Fe　balance)　was　prepared　by　using　mechanical　milling　method.　Fine　ferrite　powders　were　produced　by　oxalate　co-precipitation　process.　Flexible　composite　sheets　were　fabricated　via　tape-casting　method　by　mixing　the　flake-shape　sendust　and　various　weight　fraction　of　NiZn　ferrite.　X-ray　diffraction,　scanning　electron　microscopy　and　vibrating　sample　magnetometer　were　used　to　characterize　the　samples.　Electromagnetic　properties　measurement　results　indicated　that　permittivity,　permeability,　power　loss　of　flaky　FeSiAl/NiZn　ferrite　composite　can　be　well　tuned　by　adjusting　the　amount　of　loading　NiZn　ferrite　particles.　It　is　found　that　the　magnetic　field　coupling　efficiency　is　enhanced　by　attaching　the　composite　with　the　mix　of　ferrites.　Consequently,　the　composite　filled　with　14　wt%　of　ferrite　particles　showed　the　best　coupling　ratio　at　1　MHz-1GHz.　This　research　work　shows　promising　results　and　making　FeSiAl/NiZn　ferrite　composite　a　potential　magnetically　conductive　material　for　energy　transmission　applications,　such　as　NFC.　(C)　2017　Elsevier　B.V.　All　rights　reserved.