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In this study, the enhanced removal of cationic dye, methyl violet (MV), from aqueous solution with NaOH-modified C. camphora leaves powder (N-CLP), compared with C. camphora leaves powder (CLP), was demonstrated. Subsequently, the effects of solution pH, initial MV concentration, contact time, and temperature on the adsorption of MV by N-CLP were systematically studied. The experimental results showed that MV adsorption on N-CLP was pH-dependent and stable adsorption could be achieved at pH 4.0-10.0. Electrostatic adsorption and p-p stacking could be involved in adsorption. The adsorption process for MV on N-CLP followed pseudo-second-order kinetics model. Equilibrium adsorption data were well fitted to the Langmuir isotherm model. The adsorption process is endothermic, spontaneous and random. The adsorption property of second-regenerated N-CLP and third-regenerated N-CLP still had 0.85 times over that of N-CLP and the N-CLP could be used as a renewable bio-adsorbent for removal the refractory pollutants in wastewater.
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