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Author:

Luo, Qiang (Luo, Qiang.) | Ma, He (Ma, He.) (Scholars:马赫) | Hao, Feng (Hao, Feng.) | Hou, Qinzhi (Hou, Qinzhi.) | Ren, Jing (Ren, Jing.) | Wu, Lili (Wu, Lili.) | Yao, Zhibo (Yao, Zhibo.) | Zhou, Yu (Zhou, Yu.) | Wang, Ning (Wang, Ning.) | Jiang, Kaili (Jiang, Kaili.) | Lin, Hong (Lin, Hong.) | Guo, Zhanhu (Guo, Zhanhu.)

Indexed by:

EI Scopus SCIE

Abstract:

Organolead halide perovskite solar cells (PSC) are arising as promising candidates for next-generation renewable energy conversion devices. Currently, inverted PSCs typically employ expensive organic semiconductor as electron transport material and thermally deposited metal as cathode (such as Ag, Au, or Al), which are incompatible with their large-scale production. Moreover, the use of metal cathode also limits the long-term device stability under normal operation conditions. Herein, a novel inverted PSC employs a SnO2-coated carbon nanotube (SnO2@CSCNT) film as cathode in both rigid and flexible substrates (substrate/NiO-perovskite/Al2O3-perovskite/SnO2@CSCNT-perovskite). Inverted PSCs with SnO2@CSCNT cathode exhibit considerable enhancement in photovoltaic performance in comparison with the devices without SnO2 coating owing to the significantly reduced charge recombination. As a result, a power conversion efficiency of 14.3% can be obtained on rigid substrates while the flexible ones achieve 10.5% efficiency. More importantly, SnO2@CSCNT-based inverted PSCs exhibit significantly improved stability compared to the standard inverted devices made with silver cathode, retaining over 88% of their original efficiencies after 550 h of full light soaking or thermal stress. The results indicate that SnO2@CSCNT is a promising cathode material for long-term device operation and pave the way toward realistic commercialization of flexible PSCs.

Keyword:

perovskite solar cells charge extracting materials stabilities carbon nanotubes

Author Community:

  • [ 1 ] [Luo, Qiang]Univ Elect Sci & Technol China, State Key Lab Elect Thin Film & Integrated Device, Chengdu 610054, Sichuan, Peoples R China
  • [ 2 ] [Hao, Feng]Univ Elect Sci & Technol China, State Key Lab Elect Thin Film & Integrated Device, Chengdu 610054, Sichuan, Peoples R China
  • [ 3 ] [Hou, Qinzhi]Univ Elect Sci & Technol China, State Key Lab Elect Thin Film & Integrated Device, Chengdu 610054, Sichuan, Peoples R China
  • [ 4 ] [Ren, Jing]Univ Elect Sci & Technol China, State Key Lab Elect Thin Film & Integrated Device, Chengdu 610054, Sichuan, Peoples R China
  • [ 5 ] [Wang, Ning]Univ Elect Sci & Technol China, State Key Lab Elect Thin Film & Integrated Device, Chengdu 610054, Sichuan, Peoples R China
  • [ 6 ] [Ma, He]Beijing Univ Technol, Coll Appl Sci, Beijing 100124, Peoples R China
  • [ 7 ] [Ma, He]Tsinghua Univ, Collaborat Innovat Ctr Quantum Matter, State Key Lab Low Dimens Quantum Phys, Tsinghua Foxconn Nanotechnol Res Ctr,Dept Phys, Beijing 100084, Peoples R China
  • [ 8 ] [Jiang, Kaili]Tsinghua Univ, Collaborat Innovat Ctr Quantum Matter, State Key Lab Low Dimens Quantum Phys, Tsinghua Foxconn Nanotechnol Res Ctr,Dept Phys, Beijing 100084, Peoples R China
  • [ 9 ] [Wu, Lili]Univ Tennessee, Dept Chem & Biomol Engn, ICL, Knoxville, TN 37996 USA
  • [ 10 ] [Guo, Zhanhu]Univ Tennessee, Dept Chem & Biomol Engn, ICL, Knoxville, TN 37996 USA
  • [ 11 ] [Yao, Zhibo]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
  • [ 12 ] [Zhou, Yu]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
  • [ 13 ] [Lin, Hong]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
  • [ 14 ] [Wang, Ning]Hainan Univ, State Key Lab Marine Resource Utilizat South Chin, Haikou 570228, Hainan, Peoples R China

Reprint Author's Address:

  • [Wang, Ning]Univ Elect Sci & Technol China, State Key Lab Elect Thin Film & Integrated Device, Chengdu 610054, Sichuan, Peoples R China;;[Jiang, Kaili]Tsinghua Univ, Collaborat Innovat Ctr Quantum Matter, State Key Lab Low Dimens Quantum Phys, Tsinghua Foxconn Nanotechnol Res Ctr,Dept Phys, Beijing 100084, Peoples R China;;[Guo, Zhanhu]Univ Tennessee, Dept Chem & Biomol Engn, ICL, Knoxville, TN 37996 USA;;[Lin, Hong]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China;;[Wang, Ning]Hainan Univ, State Key Lab Marine Resource Utilizat South Chin, Haikou 570228, Hainan, Peoples R China

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Source :

ADVANCED FUNCTIONAL MATERIALS

ISSN: 1616-301X

Year: 2017

Issue: 42

Volume: 27

1 9 . 0 0 0

JCR@2022

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:287

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 139

SCOPUS Cited Count: 135

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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