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作者:

Lang, Jianlei (Lang, Jianlei.) (学者:郎建垒) | Zhou, Ying (Zhou, Ying.) | Chen, Dongsheng (Chen, Dongsheng.) (学者:陈东升) | Xing, Xiaofan (Xing, Xiaofan.) | Wei, Lin (Wei, Lin.) | Wang, Xiaotong (Wang, Xiaotong.) | Zhao, Na (Zhao, Na.) | Zhang, Yanyun (Zhang, Yanyun.) | Guo, Xiurui (Guo, Xiurui.) | Han, Lihui (Han, Lihui.) | Cheng, Shuiyuan (Cheng, Shuiyuan.) (学者:程水源)

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摘要:

Many studies have been conducted focusing on the contribution of land emission sources to PM2.5 in China; however, little attention had been paid to other contributions, especially the secondary contributions from shipping emissions to atmospheric PM2.5. In this study, a combined source apportionment approach, including principle component analysis (PCA) and WRF-CMAQ simulation, was applied to identify both primary and secondary contributions from ships to atmospheric PM2.5. An intensive PM2.5 observation was conducted from April 2014 to January 2015 in Qinhuangdao, which was close to the largest energy output port of China. The chemical components analysis results showed that the primary component was the major contributor to PM2.5, with proportions of 483%, 48.9%, 55.1% and 55.4% in spring, summer, autumn and winter, respectively. The secondary component contributed higher fractions in summer (48.2%) and winter (36.8%), but had lower percentages in spring (30.1%) and autumn (32.7%). The hybrid source apportionment results indicated that the secondary contribution (SC) of shipping emissions to PM2.5 could not be ignored. The annual average SC was 2.7%, which was comparable to the primary contribution (2.9%). The SC was higher in summer (5.3%), but lower in winter (1.1%). The primary contributions to atmospheric PM2.5 were 3.0%, 2.5%, 3.4% and 2.7% in spring, summer, autumn and winter, respectively. As for the detailed chemical components, the contributions of shipping emissions were 23%, 0.5%, 0.1%, 1.0%, 1.7% and 0.1% to elements & sea salt, primary organic aerosol (POA), element carbon (EC), nitrate, sulfate and secondary organic carbon (SOA), respectively. The results of this study will further the understanding of the implications of shipping emissions in PM2.5 pollution. (C) 2017 Elsevier Ltd. All rights reserved.

关键词:

Fine particle PCA Qinhuangdao Shipping emissions Source apportionment WRF-CMAQ

作者机构:

  • [ 1 ] [Lang, Jianlei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 2 ] [Zhou, Ying]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 3 ] [Chen, Dongsheng]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 4 ] [Xing, Xiaofan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 5 ] [Wei, Lin]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 6 ] [Wang, Xiaotong]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 7 ] [Zhao, Na]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 8 ] [Zhang, Yanyun]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 9 ] [Guo, Xiurui]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 10 ] [Han, Lihui]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 11 ] [Cheng, Shuiyuan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China

通讯作者信息:

  • 郎建垒 陈东升

    [Lang, Jianlei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China;;[Chen, Dongsheng]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China

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来源 :

ENVIRONMENTAL POLLUTION

ISSN: 0269-7491

年份: 2017

卷: 229

页码: 557-566

8 . 9 0 0

JCR@2022

ESI学科: ENVIRONMENT/ECOLOGY;

ESI高被引阀值:120

中科院分区:2

被引次数:

WoS核心集被引频次: 44

SCOPUS被引频次: 56

ESI高被引论文在榜: 0 展开所有

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中文被引频次:

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