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作者:

Zhang, J. (Zhang, J..) | Du, Y.-W. (Du, Y.-W..) | Liu, X.-J. (Liu, X.-J..) | Zhou, Y.-W. (Zhou, Y.-W..) (学者:周玉文) | Liu, C. (Liu, C..) (学者:刘超) | Yang, J.-L. (Yang, J.-L..) | Zhang, L. (Zhang, L..)

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摘要:

The application of microbubble technology for ozonation wastewater treatment could enhance ozone mass transfer, improve ozonation performance and increase ozone utilization efficiency. The ozone microbubbles were used to treat synthetic acid red 3R wastewater in the present study, and compared to ozone conventional bubbles. The ozone mass transfer and ozonation characteristics of acid red 3R were investigated when ozone microbubbles and ozone conventional bubbles were applied. The results confirmed the enhanced ozone mass transfer using microbubbles. The ozone mass transfer coefficient using microbubbles was 3.6 times higher than that using conventional bubbles under the same conditions. Simultaneously, the ozone decomposition coefficient using microbubbles was 6.2 times higher than that using conventional bubbles, which would be favorable for ·OH generation. The ozonation rate and mineralization efficiency of acid red 3R could be improved significantly using ozone microbubbles. A TOC removal efficiency of 78.0% was achieved using ozone microbubbles, which was about 2 times higher than that using ozone conventional bubbles. The ozone utilization efficiency using microbubbles was much higher that using conventional bubbles during ozonation treatment of acid red 3R. The average ozone utilization efficiencies were 97.8% and 69.3% when microbubbles and conventional bubbles were used, respectively. The oxidative ability of ozone microbubbles could be increased by enhancing ·OH generation, and as a result, the oxidative reaction of degradation intermediates was accelerated by ozone microbubbles. Especially, the mineralization ability of small organic acid intermediates using ozone microbubbles was about 1.6 times higher than that using ozone conventional bubbles. ©, 2015, Science Press. All right reserved.

关键词:

Acid red 3R; Microbubble; Mineralization; Ozonation; Ozone utilization efficiency

作者机构:

  • [ 1 ] [Zhang, J.]College of Architecture and Civil Engineering, Beijing University of Technology, Beijing, 100022, China
  • [ 2 ] [Zhang, J.]Pollution Prevention Biotechnology Laboratory of Hebei Province, School of Environmental Science and Engineering, Hebei University of Science and Technology, Shijiazhuang, 050018, China
  • [ 3 ] [Du, Y.-W.]Pollution Prevention Biotechnology Laboratory of Hebei Province, School of Environmental Science and Engineering, Hebei University of Science and Technology, Shijiazhuang, 050018, China
  • [ 4 ] [Liu, X.-J.]Pollution Prevention Biotechnology Laboratory of Hebei Province, School of Environmental Science and Engineering, Hebei University of Science and Technology, Shijiazhuang, 050018, China
  • [ 5 ] [Zhou, Y.-W.]College of Architecture and Civil Engineering, Beijing University of Technology, Beijing, 100022, China
  • [ 6 ] [Liu, C.]Pollution Prevention Biotechnology Laboratory of Hebei Province, School of Environmental Science and Engineering, Hebei University of Science and Technology, Shijiazhuang, 050018, China
  • [ 7 ] [Yang, J.-L.]Pollution Prevention Biotechnology Laboratory of Hebei Province, School of Environmental Science and Engineering, Hebei University of Science and Technology, Shijiazhuang, 050018, China
  • [ 8 ] [Zhang, L.]Pollution Prevention Biotechnology Laboratory of Hebei Province, School of Environmental Science and Engineering, Hebei University of Science and Technology, Shijiazhuang, 050018, China

通讯作者信息:

  • [Zhang, J.]College of Architecture and Civil Engineering, Beijing University of TechnologyChina

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来源 :

Environmental Science

ISSN: 0250-3301

年份: 2015

期: 2

卷: 36

页码: 584-589

被引次数:

WoS核心集被引频次: 0

SCOPUS被引频次: 7

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