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学者姓名：戴洪兴
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摘要 ：
Designing highly efficient photocatalysts is significantly important to degrade the harmful pollutions in water. In this study, photocatalyst of Fe3O4-ED-rGO with dissolved HPV was successfully prepared and electron microscopy characterization revealed that large number of single tungsten/vanadium atom oxide (ST/VAO) was homogeneously deposited on Fe3O4 nanoparticles in SMAO-MrGO-ED sample and occupied the bivalent Fe2+ sites. Meanwhile, phase analysis confirmed that the Fe3O4 nanocomposites were mostly conversed from the reducted Fe2O3 by the hydrolysis of rGO-ED-HPV. Such a highly dispersed monatomic adsorption on the bivalent Fe2+ of polycrystalline SMAO-MrGO-ED nanocomposite not only benefits for the visible light absorption from 2.7 eV to 2.10 eV, but also offers abundantly active sites to get the highest activity of 98.43% and 98.12% for ciprofloxacin (CF) and ibuprofen (IBF) photodegradation, respectively. All these discoveries give us a new insight to design the photocatalysts with high photodegradation efficiency, low cost, short reaction time and good reusability.
关键词 ：
Ciprofloxacin Ciprofloxacin Ibuprofen Ibuprofen Magnetic nanocomposite Magnetic nanocomposite Photodegradation Photodegradation Single metal atom oxide Single metal atom oxide
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| GB/T 7714 | Selvakumar, Karuppaiah , Wang, Yueshuai , Lu, Yue et al. Single metal atom oxide anchored Fe3O4-ED-rGO for highly efficient photodecomposition of antibiotic residues under visible light illumination [J]. | APPLIED CATALYSIS B-ENVIRONMENTAL , 2022 , 300 . |
| MLA | Selvakumar, Karuppaiah et al. "Single metal atom oxide anchored Fe3O4-ED-rGO for highly efficient photodecomposition of antibiotic residues under visible light illumination" . | APPLIED CATALYSIS B-ENVIRONMENTAL 300 (2022) . |
| APA | Selvakumar, Karuppaiah , Wang, Yueshuai , Lu, Yue , Tian, Bohai , Zhang, Zeyu , Hu, Jingcong et al. Single metal atom oxide anchored Fe3O4-ED-rGO for highly efficient photodecomposition of antibiotic residues under visible light illumination . | APPLIED CATALYSIS B-ENVIRONMENTAL , 2022 , 300 . |
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摘要 ：
Manganese oxide supported Pt single atoms (Pt-1/MnOx) are prepared by the molten salt method. Catalytic oxidation of toluene and iso-hexane, typical emissions from furniture paints industry, is tested. Pt-1/MnOx shows poor and high catalytic stability for toluene and iso-hexane oxidation, respectively. Enhancement in the catalytic stability for toluene oxidation is observed after the hydrogen reduction treatment of Pt-1/MnOx at 200 degrees C. The hydrogen treated catalyst possesses the weaker Mn-O bonds and lower coordination number of Pt-O, with superior mobility of lattice oxygen and appropriate toluene adsorption. Balancing lattice oxygen mobility and volatile organic compounds adsorption is important for the catalytic stability of Pt-1/MnOx. For the oxidation of toluene and iso-hexane mixture, owing to the competitive adsorption, iso-hexane oxidation is greatly inhibited, while toluene oxidation is not influenced. The present Pt-1/MnOx catalyst holds promising prospect in furniture paints industry applications because of high catalytic stability and water resistance ability.
关键词 ：
Catalytic stability Catalytic stability Lattice oxygen mobility Lattice oxygen mobility Single atom catalyst Single atom catalyst VOCs adsorption VOCs adsorption VOCs removal VOCs removal
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| GB/T 7714 | Feng, Yuan , Wang, Chongchen , Wang, Can et al. Catalytic stability enhancement for pollutant removal via balancing lattice oxygen mobility and VOCs adsorption [J]. | JOURNAL OF HAZARDOUS MATERIALS , 2022 , 424 . |
| MLA | Feng, Yuan et al. "Catalytic stability enhancement for pollutant removal via balancing lattice oxygen mobility and VOCs adsorption" . | JOURNAL OF HAZARDOUS MATERIALS 424 (2022) . |
| APA | Feng, Yuan , Wang, Chongchen , Wang, Can , Huang, Haibao , Hsi, Hsing-Cheng , Duan, Erhong et al. Catalytic stability enhancement for pollutant removal via balancing lattice oxygen mobility and VOCs adsorption . | JOURNAL OF HAZARDOUS MATERIALS , 2022 , 424 . |
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摘要 ：
A series of three-dimensionally ordered macroporous (3DOM) nickel-copper mixed oxides (with the NiO/CuO molar ratios of 3 : 3, 3 : 2, and 3 : 1) calcined at various temperatures (450, 550, and 650 degrees C) were prepared using the dual-templating (Pluronic P123 and polymethyl methacrylate (PMMA)) method in a mixed solution of ethylene glycol and methanol with different volumetric ratios (1 : 2, 1 : 1.5, and 1 : 1). The sample obtained after the use of P123 and PMMA exhibited a much higher catalytic activity for CO oxidation, over which a complete CO conversion was achieved at 138 degrees C, CO/O-2 volumetric ratio = 2 : 5, and space velocity = 60,000 mL/(g h), and this catalyst possessed good stability in the presence of water vapor in the feed stream. The large surface area, high oxygen adspecies concentration, good low-temperature reducibility, and unique nanovoid 3DOM structure were accountable for the superior catalytic performance of the sample prepared by the dual P123- and PMMA-templating method.
关键词 ：
Calcination temperature Calcination temperature CO oxidation CO oxidation Dual-templating method Dual-templating method Porous Ni-Cu oxides Porous Ni-Cu oxides Three-dimensionally ordered macropore Three-dimensionally ordered macropore
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| GB/T 7714 | Rastegarpanah, Ali , Liu, Yuxi , Deng, Jiguang et al. Influence of preparation method on catalytic performance of three-dimensionally ordered macroporous NiO-CuO for CO oxidation [J]. | JOURNAL OF SOLID STATE CHEMISTRY , 2021 , 297 . |
| MLA | Rastegarpanah, Ali et al. "Influence of preparation method on catalytic performance of three-dimensionally ordered macroporous NiO-CuO for CO oxidation" . | JOURNAL OF SOLID STATE CHEMISTRY 297 (2021) . |
| APA | Rastegarpanah, Ali , Liu, Yuxi , Deng, Jiguang , Jing, Lin , Pei, Wenbo , Zhang, Xing et al. Influence of preparation method on catalytic performance of three-dimensionally ordered macroporous NiO-CuO for CO oxidation . | JOURNAL OF SOLID STATE CHEMISTRY , 2021 , 297 . |
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摘要 ：
In this work, we constructed a red phosphorus (RP)/TiO2 composite system via a chemical vapor deposition strategy. The evolution of the fibrous phased RP nanorods on the surface of anatase TiO2 spheres was rationally adjusted by controlling the composition of precursors. The optimal RP/TiO2 composite exhibited a significantly enhanced visible-light-driven photocatalytic H2 generation rate of 681 mu mol h-1 g-1. The tightly interior surface bonding between RP and TiO2 greatly promoted the efficient charge transfer and redistribution by suppressing the charge recombination and self-trapping processes within TiO2, resulting in prolonged lifetimes of the active charges during the photocatalytic process as investigated in detailed using femtosecond time-resolved transient absorption (fs-TA) spectroscopy.
关键词 ：
Hydrogen evolution Hydrogen evolution Photocatalysis Photocatalysis Red phosphorus Red phosphorus TiO2 TiO2
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| GB/T 7714 | Li, Shuang , Ng, Yun Hau , Zhu, Ruixue et al. In situ construction of elemental phosphorus nanorod-modified TiO(2 )photocatalysts for efficient visible-light-driven H(2 )generation [J]. | APPLIED CATALYSIS B-ENVIRONMENTAL , 2021 , 297 . |
| MLA | Li, Shuang et al. "In situ construction of elemental phosphorus nanorod-modified TiO(2 )photocatalysts for efficient visible-light-driven H(2 )generation" . | APPLIED CATALYSIS B-ENVIRONMENTAL 297 (2021) . |
| APA | Li, Shuang , Ng, Yun Hau , Zhu, Ruixue , Lv, Sijie , Wu, Chunxiao , Liu, Yuxi et al. In situ construction of elemental phosphorus nanorod-modified TiO(2 )photocatalysts for efficient visible-light-driven H(2 )generation . | APPLIED CATALYSIS B-ENVIRONMENTAL , 2021 , 297 . |
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摘要 ：
The low-cost and environmentally benign elemental red phosphorus ( RP) is a new class of photocatalysts with tunable bandgaps (ca. 1.5-2.4 eV) and has a strong visible-light response. It has been considered as a promising metal-free photocatalyst for solving the energy crisis and environmental problems. Unfortunately, due to the low-charge carrier mobility, and serve charge trapping effects, its photocatalytic activity is still restricted in comparison with the traditional compound photocatalysts. Considerable efforts, such as morphology modification, cocatalysts addition, heterostructure construction, charge trapping mitigation, have been conducted to improve the photocatalytic activity of the RP photocatalysts. In this review, the physical and chemical properties and the synthetic strategies of the RP photocatalysts were summarized along with the application in environmental remediation accompanied by the photocatalytic reaction mechanism. Finally, an overview and outlook on the problems and future avenues in designing and constructing advanced RP photocatalysts were also proposed. (C) 2021 Elsevier Ltd. All rights reserved.
关键词 ：
Elemental photocatalyst Elemental photocatalyst Environmental remediation Environmental remediation Photocatalysis Photocatalysis Red phosphorus Red phosphorus
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| GB/T 7714 | Wu, Chunxiao , Jing, Lin , Deng, Jiguang et al. Elemental red phosphorus-based photocatalysts for environmental remediation: A review [J]. | CHEMOSPHERE , 2021 , 274 . |
| MLA | Wu, Chunxiao et al. "Elemental red phosphorus-based photocatalysts for environmental remediation: A review" . | CHEMOSPHERE 274 (2021) . |
| APA | Wu, Chunxiao , Jing, Lin , Deng, Jiguang , Liu, Yuxi , Li, Shuang , Lv, Sijie et al. Elemental red phosphorus-based photocatalysts for environmental remediation: A review . | CHEMOSPHERE , 2021 , 274 . |
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摘要 ：
Improved photocatalytic activities in highly ordered porous photocatalysts are often attributed to the larger surface area, higher light absorption, and suppressed charge recombination. Other underlying reasons for the improved charge transport, however, remain elusive at this stage. Herein, 3DOM BiVO4 photocatalysts are examined to understand the carrier dynamics and their effects in photocatalytic water splitting. Quantum confinement arising from the ultrathin and crystalline wall upshifted its conduction band, enabling photocatalytic proton reduction to hydrogen gas under visible-light illumination. Time-resolved microwave conductivity spectroscopy reveals its similar to 6 times higher charge mobility and longer charge diffusion length relative to the bulk counterpart. The long lifetime (similar to 360 ns) of 3DOM BiVO4 with a power-law decay suggests the improved charge separation and the formation of shallow trapping states. Further investigation by Kelvin probe force microscope discloses a built-in electric field with upward band bending from the internal wall to the interconnection part of 3DOM BiVO4.
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| GB/T 7714 | Wu, Hao , Irani, Rowshanak , Zhang, Kunfeng et al. Unveiling Carrier Dynamics in Periodic Porous BiVO4 Photocatalyst for Enhanced Solar Water Splitting [J]. | ACS ENERGY LETTERS , 2021 , 6 (10) : 3400-3407 . |
| MLA | Wu, Hao et al. "Unveiling Carrier Dynamics in Periodic Porous BiVO4 Photocatalyst for Enhanced Solar Water Splitting" . | ACS ENERGY LETTERS 6 . 10 (2021) : 3400-3407 . |
| APA | Wu, Hao , Irani, Rowshanak , Zhang, Kunfeng , Jing, Lin , Dai, Hongxing , Chung, Hoi Ying et al. Unveiling Carrier Dynamics in Periodic Porous BiVO4 Photocatalyst for Enhanced Solar Water Splitting . | ACS ENERGY LETTERS , 2021 , 6 (10) , 3400-3407 . |
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摘要 ：
The poisoning effects of alkali metals (K and Na) and alkaline earth metals (Ca and Mg) on catalytic performance of the 2Nb4Ce/Zr-PILC catalyst for the selective catalytic reduction of NOx with NH3 (NH3-SCR) were investigated, and physicochemical properties of the catalysts were characterized by means of the X-ray diffraction XRD (XRD), Brunner-Emmet-Teller (BET), hydrogen temperature-programmed reduction (H-2-TPR), X-ray Photoelectron Spectroscopy (XPS), ammonia temperature-programmed desorption (NH3-TPD), and in situ diffuse reflectance infrared Fourier transform spectroscopy (in situ DRIFTS) techniques. Doping of M (M = K, Na, Ca, and Mg) deactivated the 2Nb4Ce/Zr-PILC catalyst according to the sequence of 0.8 K > 0.8 Na > 0.8 Ca > 0.8 Mg (M/Ce molar ratio = 0.8). The characterization results showed that the decreases in redox ability, NH3 adsorption, Ce3+/Ce4+ atomic ratio, and amount of the chemisorbed oxygen (O-beta) were the important factors influencing catalytic activities of the alkali metal-and alkaline earth metal-doped samples. Consequently, compared with the Mg- and Ca-doped samples, doping of K caused the 2Nb4Ce/Zr-PILC sample to possess the lowest redox ability, NH3 adsorption, and amount of the O-beta species, which resulted in an obvious deactivation effect.
关键词 ：
alkali metal alkali metal alkaline earth metal alkaline earth metal NH3-SCR NH3-SCR poisoning poisoning selective catalytic reduction selective catalytic reduction surface acidity surface acidity
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| GB/T 7714 | Li, Chenxi , Cheng, Jin , Ye, Qing et al. Poisoning Effects of Alkali and Alkaline Earth Metal Doping on Selective Catalytic Reduction of NO with NH3 over the Nb-Ce/Zr-PILC Catalysts [J]. | CATALYSTS , 2021 , 11 (3) . |
| MLA | Li, Chenxi et al. "Poisoning Effects of Alkali and Alkaline Earth Metal Doping on Selective Catalytic Reduction of NO with NH3 over the Nb-Ce/Zr-PILC Catalysts" . | CATALYSTS 11 . 3 (2021) . |
| APA | Li, Chenxi , Cheng, Jin , Ye, Qing , Meng, Fanwei , Wang, Xinpeng , Dai, Hongxing . Poisoning Effects of Alkali and Alkaline Earth Metal Doping on Selective Catalytic Reduction of NO with NH3 over the Nb-Ce/Zr-PILC Catalysts . | CATALYSTS , 2021 , 11 (3) . |
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摘要 ：
In this work, we first used the oil-phase co-reduction strategy to synthesize the RuxMny (Mn/Ru molar ratio (y/x) = 7 : 20, 21 : 25, and 17 : 10) intermetallic compounds, then used the KIT-6-templeting method to prepare mesoporous titania (meso-TiO2), and finally used the impregnation method to generate the RuxMny/meso-TiO2 (Ru loading = 0.60-0.79 wt%) catalysts. Various techniques were used to measure physicochemical properties of the samples, and their catalytic performance was determined for methyl ethyl ketone (MEK) oxidation. It is found that the RuxMny/meso-TiO2 samples possessed a three-dimensionally ordered mesoporous structure, a surface area of 71-173 m(2)/g, and a uniform RuxMny particle size of 2.3-2.9 nm. Among all of the samples, Ru25Mn21/meso-TiO2 exhibited the best catalytic performance and good hydrothermal stability: the temperatures at MEK conversions of 10, 50, and 90 % were 131, 226, and 248 degrees C at a space velocity of 20,000 mL/(g h), with the apparent activation energy, specific reaction rate at 160 degrees C, and turnover frequency (TOF) at 160 degrees C being 73 kJ/mol, 41.73 mmol/(g(Ru) s), and 4.20 s(-1), respectively. In addition, introduction of 5 vol% moisture to the reaction system exerted a positive effect on catalytic activity of Ru/meso-TiO2 or Ru25Mn21/meso-TiO2 at higher temperatures. Such good performance of the Ru25Mn21/meso-TiO2 sample was related to its well dispersed Ru25Mn21 nanoparticles, high adsorbed oxygen species concentration, active surface lattice oxygen, high MEK adsorption capacity, good redox ability, and strong interaction between Ru25Mn21 and meso-TiO2. We propose that MEK might be oxidized by the adsorbed oxygen and/or surface lattice oxygen species via in turn formation of 2,3-butanedione, acetaldehyde, acetic acid, formaldehyde, and formic acid, all of which were finally converted to water and carbon dioxide.
关键词 ：
Methyl ethyl ketone oxidation Methyl ethyl ketone oxidation Ordered mesoporous titania Ordered mesoporous titania RuMn intermetallic compound RuMn intermetallic compound Supported RuMn catalyst Supported RuMn catalyst Volatile organic compound Volatile organic compound
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| GB/T 7714 | Wang, Jia , Dai, Lingyun , Deng, Jiguang et al. An investigation on catalytic performance and reaction mechanism of RuMn/meso-TiO2 derived from RuMn intermetallic compounds for methyl ethyl ketone oxidation [J]. | APPLIED CATALYSIS B-ENVIRONMENTAL , 2021 , 296 . |
| MLA | Wang, Jia et al. "An investigation on catalytic performance and reaction mechanism of RuMn/meso-TiO2 derived from RuMn intermetallic compounds for methyl ethyl ketone oxidation" . | APPLIED CATALYSIS B-ENVIRONMENTAL 296 (2021) . |
| APA | Wang, Jia , Dai, Lingyun , Deng, Jiguang , Liu, Yuxi , Jing, Lin , Hao, Xiuqing et al. An investigation on catalytic performance and reaction mechanism of RuMn/meso-TiO2 derived from RuMn intermetallic compounds for methyl ethyl ketone oxidation . | APPLIED CATALYSIS B-ENVIRONMENTAL , 2021 , 296 . |
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摘要 ：
SnO2 is widely used in catalysis owing to its oxygen vacancies, reducible oxygen species, and acidity. In this work, Ru nanoparticles (NPs) supported on three-dimensionally ordered macroporous (3DOM) SnO2 (xRu/3DOM SnO2, Ru loading (x) = 0.09-1.65 wt%) were fabricated via the polyvinyl alcohol-protected reduction routes, and their catalytic activities were determined for trichloroethylene (TCE) and/or toluene oxidation. It was shown that the 0.98Ru/3DOM SnO2 sample exhibited the best activity and good thermal stability, with the temperature (T-90%) and apparent activation energy at a TCE (1000 ppmv) conversion of 90% being 300 degrees C and 44 kJ/mol at space velocity = 40,000 mL/(g h), respectively. Trichloromethane, carbon tetrachloride, tetrachloroethylene, and trichloroacetaldehyde hydrate were the main intermediates in TCE oxidation. The high catalytic performance of 0.98Ru/3DOM SnO2 was attributed to the presence of hydroxyl groups adsorbed at the oxygen vacancies, strong O-2 adsorption ability, good low-temperature reducibility, and strong interaction between Ru NPs and 3DOM SnO2. In addition, a catalytic mechanism over xRu/3DOM SnO2 was proposed under dry and humid conditions. The introduction of H2O could block some of the reaction pathways from inhibiting the production of C2Cl4, reduce formation of some by-products (e.g., CH2Cl2, CH3COOH, and C2H2Cl2), promote removal of the chlorine species, and generate a greater amount of HCl and a smaller amount of Cl-2. Furthermore, introducing toluene into the TCE stream could generate smaller amounts of organic chlorine by-products and greater amounts of inorganic chlorine products (HCl and Cl-2). We are sure that this work can provide a guideline for the industrial application of supported Ru catalysts in the removal of Cl-containing volatile organic compounds. (C) 2021 Elsevier Inc. All rights reserved.
关键词 ：
Chlorine resistance Chlorine resistance Reaction intermediate Reaction intermediate Supported ruthenium catalyst Supported ruthenium catalyst Three-dimensionally ordered macroporous tin oxide Three-dimensionally ordered macroporous tin oxide Trichloroethylene oxidation Trichloroethylene oxidation
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| GB/T 7714 | Yu, Xiaohui , Dai, Lingyun , Deng, Jiguang et al. Catalytic performance and intermediates identification of trichloroethylene deep oxidation over Ru/3DOM SnO2 catalysts [J]. | JOURNAL OF CATALYSIS , 2021 , 400 : 310-324 . |
| MLA | Yu, Xiaohui et al. "Catalytic performance and intermediates identification of trichloroethylene deep oxidation over Ru/3DOM SnO2 catalysts" . | JOURNAL OF CATALYSIS 400 (2021) : 310-324 . |
| APA | Yu, Xiaohui , Dai, Lingyun , Deng, Jiguang , Liu, Yuxi , Jing, Lin , Zhang, Xing et al. Catalytic performance and intermediates identification of trichloroethylene deep oxidation over Ru/3DOM SnO2 catalysts . | JOURNAL OF CATALYSIS , 2021 , 400 , 310-324 . |
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摘要 ：
The porous carbon (CKC-X-Y, CKC is the corn kernel-derived carbon; Xis the activation temperature; and Y is the KOH/CKC mass ratio (2, 3, 4, and 5)) adsorbents were prepared from corn kernels by the KOH activation method. Textural property and oxygen functional group amount of the CKC-X-Y sample were influenced by the activator amount and activation temperature. Among the CKC-X-Y samples, the CKC-900-3 sample displayed the highest surface area (1943 m(2)/g) and the largest pore volume (1.10 cm(3)/g), whereas the CKC-900-4 sample possessed the highest amount (45.5 %) of oxygen functional groups. The CKC-900-4 sample exhibited the largest CO2 adsorption capacity (3.63 mmol/g at 25 degrees C) among all of the CKC-X-Y samples. The results indicate that the activated corn-derived porous biochar with a high surface area and a high oxygen functional groups amount possessed a large CO2 uptake. In addition, the CKC-X-Y samples showed high CO2/N-2 selectivity, good recyclability, and easy regeneration behavior. The adsorption of CO2 was physically and chemically adsorbed on the surface of the CKC-X-Y samples, with the physical adsorption being dominant. In which CO2 was mainly chemically adsorbed on the samples with hydroxyl groups.
关键词 ：
Adsorption kinetics Adsorption kinetics Adsorption mechanism Adsorption mechanism Carbon dioixde uptake Carbon dioixde uptake Corn kernel-derived porous carbon Corn kernel-derived porous carbon Oxygen functional group Oxygen functional group
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| GB/T 7714 | Wu, Runping , Ye, Qing , Wu, Kai et al. Highly efficient CO2 adsorption of corn kernel-derived porous carbon with abundant oxygen functional groups [J]. | JOURNAL OF CO2 UTILIZATION , 2021 , 51 . |
| MLA | Wu, Runping et al. "Highly efficient CO2 adsorption of corn kernel-derived porous carbon with abundant oxygen functional groups" . | JOURNAL OF CO2 UTILIZATION 51 (2021) . |
| APA | Wu, Runping , Ye, Qing , Wu, Kai , Wang, Lanyang , Dai, Hongxing . Highly efficient CO2 adsorption of corn kernel-derived porous carbon with abundant oxygen functional groups . | JOURNAL OF CO2 UTILIZATION , 2021 , 51 . |
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