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新型环保煤尘抑尘剂的制备及其应用
期刊论文 | 2021 , 47 (6) , 57-65 | 中国煤炭
摘要&关键词 引用

摘要 :

为了有效控制煤尘大气污染和解决农业废弃物再利用的问题,以农业废弃物为原料制备环保抑尘剂并应用于煤尘控制,实现以废治污的目的.该抑尘剂以秸秆酶解液为主要原料,考察了辅料粘结剂、保湿剂和表面活性剂对抑尘剂性能的影响.研究中通过单因素实验确定出粘结剂瓜尔豆胶、阴离子表面活性剂十二烷基硫酸钠(K 12)和保湿剂乳酸钠的比例范围,并通过正交实验的方法优化了抑尘剂配方,所制得的抑尘剂在黏度和溶液的润湿性上可以表现出更优异的抑尘性能,优化配方后抑尘剂的黏度为5.8 mPa?s、表面张力为31.20 mN/m、接触角为15.2°,具有较好的润湿性能;在8 m/s的模拟风速条件下,2 h内可保持100%的抑尘效率,可以实现有效抑制煤尘的作用.煤场实际应用结果表明,使用抑尘剂后可使煤场的PM10浓度由145.2 mg/m3降至环境背景浓度,可以达到有效抑制风力扬尘的效果.

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GB/T 7714 梁文俊 , 兰童 , 张志学 et al. 新型环保煤尘抑尘剂的制备及其应用 [J]. | 中国煤炭 , 2021 , 47 (6) : 57-65 .
MLA 梁文俊 et al. "新型环保煤尘抑尘剂的制备及其应用" . | 中国煤炭 47 . 6 (2021) : 57-65 .
APA 梁文俊 , 兰童 , 张志学 , 任思达 , 王艳磊 . 新型环保煤尘抑尘剂的制备及其应用 . | 中国煤炭 , 2021 , 47 (6) , 57-65 .
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新工科视角下环境类专业学位课教学改革探索
期刊论文 | 2021 , (32) , 47-50 | 教育教学论坛
摘要&关键词 引用

摘要 :

随着世界范围内新一轮科技革命和信息产业技术革命的发展,新型教育技术如雨后春笋般步入课堂,正引领我国高等教育步入崭新的阶段.针对环境类专业学位课"大气污染控制工程"教学中的一些问题,根据课程的特点,加强课程群建设,将理论和实践教学相结合,打造智慧课堂,促进师生互动,提升教学质量,培养学生的实践能力、思维创新能力、将所学知识融会贯通并综合运用的能力,以符合新工科人才培养需求,实现工程应用型人才培养的教育目标.

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GB/T 7714 梁文俊 , 刘佳 , 李坚 . 新工科视角下环境类专业学位课教学改革探索 [J]. | 教育教学论坛 , 2021 , (32) : 47-50 .
MLA 梁文俊 et al. "新工科视角下环境类专业学位课教学改革探索" . | 教育教学论坛 32 (2021) : 47-50 .
APA 梁文俊 , 刘佳 , 李坚 . 新工科视角下环境类专业学位课教学改革探索 . | 教育教学论坛 , 2021 , (32) , 47-50 .
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基于雨课堂的“大气污染控制工程”线上线下混合教学模式初探
期刊论文 | 2021 , 8 (12) , 25-27 | 教育现代化
摘要&关键词 引用

摘要 :

摘?要:新型信息技术的迅猛发展给我国高等教育带来了改革契机,传统课堂教学向智慧课堂发展,混合式教学模式应运而生,为课堂教学的创新提供新的思路。大气污染控制工程课程是面向环境工程专业学生开设的一门重要专业学位课,主要目的是培养学生运用所学的知识能够对实际问题具有认识、分析和解决的能力。本文围绕大气污染控制工程课程教学,详细介绍了采用“雨课堂”的线上线下混合教学模式。根据当前教学改革的发展的趋势,应用“雨课堂”教学工具,从教学过程、教学手段和教学效果三个方面总结了应用“雨课堂”混合式教学的经验,旨在提高专业课程的教学效果,增加学生综合学习及运用专业知识的能力。本文可为高校专业课程的教学改革提供借鉴。

关键词 :

关键词大气污染控制工程 关键词大气污染控制工程 混合教学模式 混合教学模式 线上线下 线上线下 雨课堂 雨课堂

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GB/T 7714 梁文俊 , 刘佳 , 宋丽云 et al. 基于雨课堂的“大气污染控制工程”线上线下混合教学模式初探 [J]. | 教育现代化 , 2021 , 8 (12) : 25-27 .
MLA 梁文俊 et al. "基于雨课堂的“大气污染控制工程”线上线下混合教学模式初探" . | 教育现代化 8 . 12 (2021) : 25-27 .
APA 梁文俊 , 刘佳 , 宋丽云 , 樊星 , 李坚 . 基于雨课堂的“大气污染控制工程”线上线下混合教学模式初探 . | 教育现代化 , 2021 , 8 (12) , 25-27 .
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Application of an Asterisk Plate in the Flow Diversion of the Volatile Organic Compound Removal System SCIE
期刊论文 | 2021 , 147 (12) | JOURNAL OF ENVIRONMENTAL ENGINEERING
WoS核心集被引次数: 1
摘要&关键词 引用

摘要 :

In order to reduce process complexity and manufacturing difficulty, we proposed to use a single air distribution plate to guide the flow and achieve uniform air distribution. We established a three-dimensional model with a size ratio of 1:1 to simulation flow pattern. The optimization results revealed that it is feasible to implement our assumption. After the asterisk plate's optimization, the area uniformity index in the catalytic section was maintained above 0.92 with a maximum value of 0.95, the relative standard deviation was lower than 0.2, and the minimum value was 0.123; and the pressure drop was less than 3.00 Pa, which is in line with the actual use requirements. Among them, Asterisk I with a 30 mm thickness and 15 mm right shift has the best optimization effect. (c) 2021 American Society of Civil Engineers.

关键词 :

CFD modeling CFD modeling Deflector Deflector Optimization Optimization VOC removal system VOC removal system

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GB/T 7714 Liang, Wen-Jun , Ju, Hao-Lin , Ren, Si-da et al. Application of an Asterisk Plate in the Flow Diversion of the Volatile Organic Compound Removal System [J]. | JOURNAL OF ENVIRONMENTAL ENGINEERING , 2021 , 147 (12) .
MLA Liang, Wen-Jun et al. "Application of an Asterisk Plate in the Flow Diversion of the Volatile Organic Compound Removal System" . | JOURNAL OF ENVIRONMENTAL ENGINEERING 147 . 12 (2021) .
APA Liang, Wen-Jun , Ju, Hao-Lin , Ren, Si-da , Li, Xiang . Application of an Asterisk Plate in the Flow Diversion of the Volatile Organic Compound Removal System . | JOURNAL OF ENVIRONMENTAL ENGINEERING , 2021 , 147 (12) .
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Preparation and optimization of the environmental dust suppressant with agricultural waste straw SCIE
期刊论文 | 2021 | ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
WoS核心集被引次数: 4
摘要&关键词 引用

摘要 :

In order to reduce the dust pollution caused by the coal mining process, a novel composite environmental dust suppressant for coal dust control was synthesized by corn straw, sodium carboxymethyl cellulose (CMC), and additives. This study focused on the preparation conditions of the dust suppressant, and the performances of which were investigated systematically. Response surface method (RSM) was used to optimize the raw material formulation and preparation parameters. The optimum mass ratio of straw, CMC, and alkali of the dust suppression was 65:20:15 (m/m), which was prepared under the conditions of the reaction time being 1.5 h and the rotation speed being 300 r/min. The pH of the dust suppressant was 8.0, and the state of which was suspension. Additives were benefited to enhance the suppressant performance, and the surface tension and the contact angle could decrease to 32.4 mN/m and 32.0 degrees. The suppressant has a maximum viscosity of 363.6 mPa center dot s, and the compressive strength could be up to 200 kPa. The hygroscopic rate could reach more than 4%. The wind erosion resistance could be up to 99 % at the wind speed of 14 m/s. After spraying the dust suppressant, the gap between particles was filled with dust suppressant, and the adjacent particles were bound by strong mechanical action.

关键词 :

Agricultural waste Agricultural waste Dust suppressant Dust suppressant Environmental friendly Environmental friendly Straw Straw

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GB/T 7714 Liang, Wenjun , Zhang, Zhixue , Chi, Hao et al. Preparation and optimization of the environmental dust suppressant with agricultural waste straw [J]. | ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH , 2021 .
MLA Liang, Wenjun et al. "Preparation and optimization of the environmental dust suppressant with agricultural waste straw" . | ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH (2021) .
APA Liang, Wenjun , Zhang, Zhixue , Chi, Hao , Ren, Sida . Preparation and optimization of the environmental dust suppressant with agricultural waste straw . | ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH , 2021 .
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Use of rare earth elements in single-atom site catalysis: A critical review - Commemorating the 100th anniversary of the birth of Academician Guangxian Xu SCIE CSCD
期刊论文 | 2021 , 39 (3) , 233-242 | JOURNAL OF RARE EARTHS
WoS核心集被引次数: 18
摘要&关键词 引用

摘要 :

Rare earth metals are strategic resources with potential applications in optics, metallurgy and catalysis. In recent years, single-atom site catalysts (SASCs) have attracted increasing attention owing to their 100% atom efficiency and unique catalytic performances. Over the past decade, rare earth elements, including rare earth metals and their oxides, have shown great potential in SASCs. However, systematic analyses of data are still handful. In this mini-review, the use of rare earth metals and their oxides in SASCs was summarized and the results are discussed. A particular focus was paid to the synthetic strategies, characterization of rare earth-containing SASCs, and applications as catalysis supports, promoters and active sites. Current issues faced by rare-earth metals and their oxides in SASCs, as well as future prospects were also provided. (C) 2020 Chinese Society of Rare Earths. Published by Elsevier B.V. All rights reserved.

关键词 :

Applications Applications Characterization Characterization Rare earth catalysis Rare earth catalysis Single-atom site catalysis Single-atom site catalysis Synthetic strategies Synthetic strategies

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GB/T 7714 Zhang, Ningqiang , Yan, Han , Li, Lingcong et al. Use of rare earth elements in single-atom site catalysis: A critical review - Commemorating the 100th anniversary of the birth of Academician Guangxian Xu [J]. | JOURNAL OF RARE EARTHS , 2021 , 39 (3) : 233-242 .
MLA Zhang, Ningqiang et al. "Use of rare earth elements in single-atom site catalysis: A critical review - Commemorating the 100th anniversary of the birth of Academician Guangxian Xu" . | JOURNAL OF RARE EARTHS 39 . 3 (2021) : 233-242 .
APA Zhang, Ningqiang , Yan, Han , Li, Lingcong , Wu, Rui , Song, Liyun , Zhang, Guizhen et al. Use of rare earth elements in single-atom site catalysis: A critical review - Commemorating the 100th anniversary of the birth of Academician Guangxian Xu . | JOURNAL OF RARE EARTHS , 2021 , 39 (3) , 233-242 .
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Performance and poisoning analysis of organic sulfur resistance of Pd-Ce catalyst in catalytic oxidation of VOCs SCIE
期刊论文 | 2021 , 9 (6) | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING
WoS核心集被引次数: 26
摘要&关键词 引用

摘要 :

In this paper, the effect of organic sulfur on the catalytic oxidation of toluene was explored. It was found that the low concentration of organic sulfur could cause rapid deactivation of the catalyst, and the activity of the catalyst could be restored to 100% after stopping the application of sulfur. The sulfation modification could significantly improve the organic sulfur resistance of the catalyst by changing the support and the sulfation modification of the support. There was a large amount of carbon deposition and a small amount of S-containing substances on the catalyst surface after the introduction of organic sulfur through the methods of TG, BET, FTIR, SEM (Mapping) and XPS. Then, through in-situ DRIFT and CH3SH-TPD, it was found that sulfation modification could inhibit the adsorption of organic sulfur on the catalyst surface and reduce the competitive adsorption. The decrease of catalyst efficiency due to the presence of organic sulfur in the reaction gas during VOCs catalytic oxidation is mainly due to the competitive adsorption of organic sulfur and VOCs molecules, and the temperature of VOCs catalytic oxidation of organic sulfur. Some polyhydrocarbons, ethyl sulfide, dimethyl sulfoxide and other substances were produced by incomplete oxidation, which covered the surface of the catalyst due to adsorption or deposition, resulting in catalyst poisoning.

关键词 :

Catalytic oxidation Catalytic oxidation Organic sulfur Organic sulfur Poison mechanism Poison mechanism VOCs VOCs

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GB/T 7714 Ren, Sida , Liang, Wenjun , Fang, Hongping et al. Performance and poisoning analysis of organic sulfur resistance of Pd-Ce catalyst in catalytic oxidation of VOCs [J]. | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING , 2021 , 9 (6) .
MLA Ren, Sida et al. "Performance and poisoning analysis of organic sulfur resistance of Pd-Ce catalyst in catalytic oxidation of VOCs" . | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING 9 . 6 (2021) .
APA Ren, Sida , Liang, Wenjun , Fang, Hongping , Zhu, Yuxue . Performance and poisoning analysis of organic sulfur resistance of Pd-Ce catalyst in catalytic oxidation of VOCs . | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING , 2021 , 9 (6) .
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Catalytic combustion of chlorobenzene at low temperature over Ru-Ce/TiO2: High activity and high selectivity SCIE
期刊论文 | 2021 , 623 | APPLIED CATALYSIS A-GENERAL
WoS核心集被引次数: 21
摘要&关键词 引用

摘要 :

Ru/TiO2 and Ru-Ce/TiO2 catalysts were prepared by the equal-volume impregnation method to test their catalytic oxidation of chlorobenzene(CB), with the aim to investigate the effect of Ce addition on the redox capacity of the catalysts under the premise of reducing the content of noble metals. It was found that the introduction of Ce conserved the high catalytic efficiency of the catalyst while reducing the content of noble metal, and the catalysis of CB was greatly improved at low temperatures. Compared with the 0.4Ru/TiO2 catalyst, the T-10 and T-90 of the 0.4Ru-1.0Ce/TiO2 catalyst decreased by 50 degrees C and 60 degrees C respectively. It presented high reaction rate at 170. with an increase from 1.21 x 10(-8) mol/min.m(2) for the 0.4Ru/TiO2 catalyst to 10.45 x 10(-8) mol/min.m(2), making it even better than the 2.0Ru/TiO2 catalyst. The structure and morphology of the Ru/TiO2 catalyst did not change with the Ce doping and the mesoporous structure of the catalysts was maintained. CeO2 can not only store and release oxygen, but also improve the activity and dispersion of precious metal loaded. The formation of Ru-O-Ce under the interaction between CeO2 and Ru species promoted electron transfer and improved the mobility of surface oxygen, thus forming RuOx with higher valance. The introduction of Ce improved the yield of COx and selectivity towards inorganic chlorine (HCl and Cl-2) and prevented the catalyst from producing more chlorinated by-products, thus greatly reducing the chance of producing more toxic dioxins.

关键词 :

Catalytic oxidation Catalytic oxidation Cerium Cerium Chlorobenzene Chlorobenzene Ru-Ce/TiO2 Ru-Ce/TiO2 Ruthenium Ruthenium

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GB/T 7714 Liang, Wenjun , Zhu, Yuxue , Ren, Sida et al. Catalytic combustion of chlorobenzene at low temperature over Ru-Ce/TiO2: High activity and high selectivity [J]. | APPLIED CATALYSIS A-GENERAL , 2021 , 623 .
MLA Liang, Wenjun et al. "Catalytic combustion of chlorobenzene at low temperature over Ru-Ce/TiO2: High activity and high selectivity" . | APPLIED CATALYSIS A-GENERAL 623 (2021) .
APA Liang, Wenjun , Zhu, Yuxue , Ren, Sida , Li, Qinglei , Song, Liyun , Shi, Xiujuan . Catalytic combustion of chlorobenzene at low temperature over Ru-Ce/TiO2: High activity and high selectivity . | APPLIED CATALYSIS A-GENERAL , 2021 , 623 .
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工业炉窑VOCs废气吸附-脱附-催化一体化净化技术研究
期刊论文 | 2020 , 26 (05) , 48-55 | 洁净煤技术
摘要&关键词 引用

摘要 :

针对小型企业工业炉窑VOCs低浓度、不连续的排放特点,以商用活性炭为吸附材料,采用自制Pd-Ce/Al_2O_3双元催化剂开展工业炉窑VOCs废气吸附-脱附-催化一体化净化技术研究,通过BET、SEM和TG表征手段对吸脱附再生前后的活性炭进行表征测试。以甲苯为探针分子,考察不同脱附时间、烟气稀释倍数、催化温度及烟气循环次数对该工艺净化甲苯废气性能的影响。研究表明100℃下热脱附1 h即可将吸附物质基本脱除,催化温度为320℃时,甲苯即可完全催化氧化;系统循环操作10~15次后,活性炭材料在100℃下焙烧6 h进行彻底再生,具有最好的经济效益。表征结果表明,经多次热再生后,活性炭孔道存在部分坍塌...

关键词 :

一体化净化 一体化净化 VOCs VOCs 工业炉窑 工业炉窑 活性炭 活性炭 循环再生 循环再生

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GB/T 7714 任思达 , 梁文俊 , 张依铭 et al. 工业炉窑VOCs废气吸附-脱附-催化一体化净化技术研究 [J]. | 洁净煤技术 , 2020 , 26 (05) : 48-55 .
MLA 任思达 et al. "工业炉窑VOCs废气吸附-脱附-催化一体化净化技术研究" . | 洁净煤技术 26 . 05 (2020) : 48-55 .
APA 任思达 , 梁文俊 , 张依铭 , 李庆磊 , 朱玉雪 . 工业炉窑VOCs废气吸附-脱附-催化一体化净化技术研究 . | 洁净煤技术 , 2020 , 26 (05) , 48-55 .
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低温等离子体协同催化降解甲苯生成副产物臭氧的影响因素 CSCD
期刊论文 | 2020 , 39 (07) , 2893-2899 | 化工进展
CNKI被引次数: 1
摘要&关键词 引用

摘要 :

低温等离子体协同催化降解甲苯过程中,在降解污染物的同时活性氧原子聚合生成臭氧。本文研究比较了不同催化剂、放电能量水平、催化段长度和气速条件下的臭氧浓度变化和甲苯降解情况,探究了低温等离子体协同催化降解甲苯过程中臭氧的生成情况。研究表明,将7.5%Mn/堇青石催化剂置于放电区时能有效抑制臭氧生成,促进甲苯降解,提高系统能效,臭氧最高浓度相比无催化剂时降低63.32mg/m~3;而0.2%Pd-0.3%Ce/堇青石催化剂对甲苯降解和抑制臭氧的性能较差。随着系统能量水平的提高,甲苯降解率和臭氧生成浓度逐渐升高。臭氧生成浓度与催化段长度呈正相关关系,与气速的关系则相反。在不同的外加电压条件下,臭氧生成...

关键词 :

催化氧化 催化氧化 臭氧 臭氧 甲苯 甲苯 低温等离子体 低温等离子体

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GB/T 7714 梁文俊 , 孙慧频 , 朱玉雪 et al. 低温等离子体协同催化降解甲苯生成副产物臭氧的影响因素 [J]. | 化工进展 , 2020 , 39 (07) : 2893-2899 .
MLA 梁文俊 et al. "低温等离子体协同催化降解甲苯生成副产物臭氧的影响因素" . | 化工进展 39 . 07 (2020) : 2893-2899 .
APA 梁文俊 , 孙慧频 , 朱玉雪 , 任思达 . 低温等离子体协同催化降解甲苯生成副产物臭氧的影响因素 . | 化工进展 , 2020 , 39 (07) , 2893-2899 .
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